and elemen tal analysis and crystallographic structure determination where possible) and their excited state properties have been probed using photophysical methods (including room and low temperature UV vis absorption and fluorescence spectroscopy and fluoresence quantum yields and lifetime). Ab initio calculations have afforded opti mised geometries which have been compared to molecular structures determined us ing X ray diffraction and vibrational spectroscopy. TD DFT calculations have been used to rationalise the observed photophysical spectra
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